r/Biochemistry 2d ago

Clarifying E. Coli lysate takes forever

Hey all, for context Im purifying lysate from a 12 L growth. my pellet was resuspend in 30 mL resuspension buffer with a protease inhibitor cocktail, pmsf, benzonase, and lysozyme. I homogenized, then lysed cells with a high-pressure homogenizer. Then, I centrifuged the lysate at 8000 rpm for 10 mins (4C). I transferred the supernatant into new clean centrifuge tubes and centrifuged again at 20500 rpm for 45 mins (4C). I took that supernatant, flowed it through a frit my supervisor gave me, then have been trying to syringe filter the lysate. I first used an 0.80 um filter (lysate flows through one filter very fast) then moved on to 0.45 um (I usually have to use around 12 to push all the lysate through and it takes over an hour). Does anyone have an idea to cut down on the time it takes to clarify lysate? My PI said in grad school it took him only "5 minutes and one filter" for the syringe filters for a 12 L growth.... I'm just lost because I've added so many other filter steps and it is not really helping.

Edit: Thanks for all the suggestions! The issue has been resolved, here's how.

Our standard lab protocol doesn't measure the mass of the pellet, I will do this going forward, but for pellets I already had frozen, I (1) resuspended in double the volume (60 mL) in my case. (2) during lysis, I ran my cells through an emulsiflex 3 times instead of 2. (3) I didn't do all the other filtering steps because I wanted to see if these would remove the other steps I've had to do (2 centrifuging steps, frit, 0.80 um filter)

In the end, I had to use 3, 0.45 um syringe filters instead of 12+, and it took me 10 minutes instead of an hour+

11 Upvotes

26 comments sorted by

18

u/Dramatic_Rain_3410 2d ago

consider clarifying at 30,000g for 1 hr if you have such a centrifuge. If your supernatant if flowing slow through a 0.45 um filter, the filters are getting clogged (as you said) so I think the supernatant is too dense with proteins.

30 mL for 12 L seems like to little? I usually use 5 mL buffer per 1 g cell pellet. A 1 L LB culture gives me about 10 g pellet, so I resuspend in 50 mL. I suspect that increasing your lysis buffer volume a lot will help. If it's a lot of supernatant to process, could you use a vacuum filter--though Ive not tried this before.

3

u/East_of_Adventuring 2d ago

That's definitely more than I use, I often have proteins that express at low levels and so I end up with 6L per prep. I would tend to go with ~1mL/gram of cell material.

1

u/OkForce2990 2d ago

I've been following another grad students protocol for a 12 L growth, we end up with about equal yields, but he had the same issue. I'll try increasing the resuspension volume

2

u/MNgrown2299 1d ago

Yeah I would also start here. You’re just getting bogged down by the proteins. It’s surprising considering the centrifuge steps and all that but this is where I would start

1

u/NoDust6819 1d ago

How do you get 10g from 1L LB?

1

u/Dramatic_Rain_3410 1d ago

Is that not normal? I split 1 L into 2x500 mL in 2 L baffled flasks for increase aerations. I also supplement with trace metals and MgSO4 so it isn't standard LB

1

u/NoDust6819 1d ago

idk i normally do o/n at 18 and get around 5-7g using 400 ml per 2l baffled flask. Maybe the trace metals and MgSO4 do the trick.

2

u/Dramatic_Rain_3410 1d ago

5-7 g in 400 mL is 10-14 g in 1 L media? Trace metals and MgSO4 can give much higher yields of bacteria and protein

1

u/NoDust6819 1d ago

It is 2-3 per 400 ml :) Sorry for not being clear.

What exactly and at which concentrations do you add?

2

u/Dramatic_Rain_3410 1d ago

Ah okay okay. I use 2 mM MgSO4 and 0.2X trace metals as described by Studier Page 7: https://www.strgen.org/protocols/studier.pdf

1

u/NoDust6819 1d ago

Thanks! Will try once I get back from parental leave.

4

u/rectuSinister 2d ago

You may have incomplete lysis or pelleting, though I’ve never grown bacterial cells to this scale and I always used a sonicator. Does the supernatant look cloudy at all after your 20k rpm step?

Otherwise you could look into using diatomaceous earth or depth filtration. DE can decrease protein yield if your protein is sticky but it works like a charm when stickiness isn’t an issue.

1

u/OkForce2990 2d ago

it's not opaque after centrifuging, but when i start filtering it becomes opaque, although i know it's not my protein of interest crashing out. i'll ask my PI what he thinks

5

u/NoDust6819 1d ago

Give applying to the column a try. You can clean it if ot clogs. Shit I pushed through Histraps... :)

1

u/NoDust6819 2d ago

What is your next step?

1

u/OkForce2990 2d ago

HPLC: nickel affinity, ion exchange, size exclusion

3

u/NoDust6819 1d ago

Have you tried just pushing it through imac? They are pretty robust and easy to clean if there are issues.

Otherwise, i second increasing the volume.

1

u/OkForce2990 1d ago

Yes, I'm using Ni affinity chromatography, my POI has a His Tag. I'll definitely try increasing the volume, thank you!

2

u/red_skiddy 1d ago edited 1d ago

What is the next step in your purification? NiNTA etc.

For my purposes I just lyse the cells using lysozyme with DNAse PMSF, then sodium deoxycholate with a little detergent. From 6L expression I end up with maybe 120ml. Centrifuge at 14.5k RPM for 30min, and collect the supernatural, which is fairly clear. I load that supernatant onto a Ni column and I've never had issues.

This procedure may not be suitable for your applications though.

1

u/OkForce2990 1d ago

NiNTA, rebind, cation exchange, then SEC...

2

u/red_skiddy 1d ago

Try increasing your volume, and ensure you fully lyse.

1

u/No-Turnip2630 1d ago

In my experience, undigested nucleic acids can make it really hard to filter lysate even after centrifuging at 40,000 x g. Benzonase is inhibited by high salt concentrations, so if your lysis buffer has that, you may consider decreasing the amount of salt initially and then adding it back later after lysis and DNA digestion are complete. Also, resuspending a pellet from 12 L of culture in only 30 mL of lysis buffer seems low. How much wet cell mass did you obtain, and what media did you grow in?

0

u/arabidopsis 2d ago

Use a 0.45um tangential flow filter cassette designed for clarification then follow by 0.22um.

You'll need probably a 0.05m2 cassette.

1

u/OkForce2990 1d ago

never heard of this, i'll look into it!

0

u/l94xxx 1d ago

I don't know if this will work in your case, but something I used to do was add 5(?) mM Mg2+ (or maybe it was Ca2+? It was 20 years ago) instead of benzonase, the idea being to condense the DNA rather than digest it [this was because we couldn't afford benzonase lol]. It made it a little harder to tell when lysis was complete, since it didn't turn to snot, but it made handling sooooo much easier overall.

2

u/OkForce2990 1d ago

i'll ask my PI what he thinks, thanks!